J. Phys. Soc. Jpn. 74 (2005) pp. 445-449 |Next Article| |Table of Contents|
|Full Text PDF (188K)| |Buy This Article|
Soft Phonons and Structural Phase Transitions in La1.875Ba0.125CuO4
Hiroyuki Kimura,
Yukio Noda,
Hideto Goka1,
Masaki Fujita2,
Kazuyoshi Yamada2 and
Gen Shirane3
Institute of Multidisciplinary Research for Advanced Materials, Tohoku University, Sendai 980-8577
1Institute for Chemical Research, Kyoto University, Gokasho, Uji, Kyoto 610-0011
2Institute of Material Research, Tohoku University, Sendai 980-8577
3Department of Physics, Brookhaven National Laboratory, Upton, NY 11973-5000, U.S.A.
(Received October 5, 2004)
Soft phonon behavior associated with a structural phase transition from the low-temperature-orthorhombic (LTO) phase (Bmab symmetry) to the low-temperature-tetragonal (LTT) phase (P42/ncm symmetry) was investigated in La1.875Ba0.125CuO4 using neutron scattering. As temperature decreases, the TO-mode at Z-point softens and approaches to zero energy around Td2=62 K, where the LTO–LTT transition occurs. Below Td2, the phonon hardens quite rapidly and its energy almost saturates below 50 K. At Td2, the energy dispersion of the soft phonon along in-plane direction significantly changes while the dispersion along out-of-plane direction is almost temperature independent. Coexistence between the LTO phase and the LTT phase, seen in both the soft phonon spectra and the peak profiles of Bragg reflection, is discussed in context of the order of structural phase transitions.
©2005 The Physical Society of Japan
URL:
http://jpsj.ipap.jp/link?JPSJ/74/445/
DOI: 10.1143/JPSJ.74.445
- A. R. Moodenbaugh, Y. Xu, M. Suenaga, T. J. Follcerts and R. N. Shelton:
Phys. Rev. B 38 (1988) 4596[APS].
- J. D. Axe, A. H. Moudden, D. Hohlwein, D. E. Cox, K. M. Mohanty, A. R. Moodenbaugh and Y. Xu:
Phys. Rev. Lett. 62 (1989) 2751[APS].
- M. K. Crawford, R. L. Harlow, E. M. McCarron, W. E. Farneth, J. D. Axe, H. Chou and Q. Huang:
Phys. Rev. B 44 (1991) 7749[APS].
- R. J. Birgeneau, C. Y. Chen, D. R. Gabbe, H. P. Jenssen, M. A. Kastner, C. J. Peters, P. J. Picone, T. Thio, T. R. Thurston, H. L. Tuller, J. D. Axe, P. Böni and G. Shirane:
Phys. Rev. Lett. 59 (1987) 1329[APS].
- P. Böni, J. D. Axe, G. Shirane, R. J. Birgeneau, D. R. Gabbe, H. P. Jenssen, M. A. Kastner, C. J. Peters, P. J. Picone and T. R. Thurston:
Phys. Rev. B 38 (1988) 185[APS].
- T. R. Thurston, R. J. Birgeneau, D. R. Gabbe, H. P. Jenssen, M. A. Kastner, P. J. Picone, N. W. Preyer, J. D. Axe, P. Böni, G. Shirane, M. Sato, K. Fukuda and S. Shamoto:
Phys. Rev. B 39 (1989) 4327[APS].
- B. Keimer, R. J. Birgeneau, A. Cassanho, Y. Endoh, M. Greven, M. A. Kastner and G. Shirane:
Z. Phys. B 91 (1993) 373[CrossRef].
- Q1 and Q2 corresponds to displacements perpendicular to a- and b-axis in the LTO phase, which arises from the tilting of CuO6 octahedra. Q can be defined as the vectorial sum of Q1 and Q2 with phase angle θ. In this definition, θ can be regarded as the angle between a-axis of the LTO phase and the tilt axis of CuO6 octahedra, and Q corresponds to the rotation amplitude around the tilt axis.
- M. Braden, O. Hoffels, W. Schnelle, B. Büchner, G. Heger, B. Hennion, I. Tanaka and H. Kojima:
Phys. Rev. B 47 (1993) 12288[APS].
- C. H. Lee, K. Yamada, M. Arai, S. Wakimoto, S. Hosoya and Y. Endoh:
Physica C 257 (1996) 264[CrossRef].
- H. Kimura, K. Hirota, C. H. Lee, K. Yamada and G. Shirane:
J. Phys. Soc. Jpn. 69 (2000) 851[JPSJ].
- J. M. Tranquada, B. J. Sternlieb, J. D. Axe, Y. Nakamura and S. Uchida:
Nature 375 (1995) 561[CrossRef].
- J. M. Tranquada, J. D. Axe, N. Ichikawa, Y. Nakamura, S. Uchida and B. Nachumi:
Phys. Rev. B 54 (1996) 7489[APS].
- M. Fujita, H. Goka, K. Yamada, J. M. Tranquada and L. P. Regnault:
to be published in Phys. Rev. B (cond-mat/0403396[e-print arXiv]).
- S. J. L. Billinge, G. H. Kwei, A. C. Lawson and J. C. Thompson:
Phys. Rev. Lett. 71 (1993) 1903[APS].
- W. Ting, K. Fossheim and T. Lægreid:
Solid State Commun. 75 (1990) 727[CrossRef].